Nonlinear Absorption and Photoluminescence of CdTe Nanotetrapods with CdSe Tips under Nonresonance Excitation of Excitons

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Abstract

The nonlinear absorption and photoluminescence of CdTe/CdSe nanotetrapod colloids have been studied by the pump–probe method for the case of single-photon nonresonance excitation of excitons. A competition between the short-wave and long-wave shifts of the peak of photoluminescence associated with an indirect electron–hole transition, which is observed with increasing excitation radiation intensity, has been found and explained. The former shift is associated with an increase in the one-dimensional exciton radius after the exciton state occupation, and the latter shift may be attributed to the charge-induced Stark effect and local heating of nanotetrapods as a result of electron–phonon interaction at nonresonance excitation of the system.

About the authors

S. Yu Gavrilov

Moscow State University, Faculty of Physics

Email: logbook1@yandex.ru
119991, Moscow, Russia

A. M Smirnov

Moscow State University, Faculty of Physics; Kotel’nikov Institute of Radio Engineering and Electronics, Russian Academy of Sciences

Email: logbook1@yandex.ru
119991, Moscow, Russia; 125009, Moscow, Russia

M. V Kozlova

Moscow State University, Faculty of Materials Science

Email: logbook1@yandex.ru
119991, Moscow, Russia

R. B Vasil'ev

Moscow State University, Faculty of Physics

Email: logbook1@yandex.ru
119991, Moscow, Russia

V. S Dneprovskiy

Moscow State University, Faculty of Materials Science

Author for correspondence.
Email: logbook1@yandex.ru
119991, Moscow, Russia

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